Article citationsMore>>
Darby, S., Hill, D., Auvinen, A., Barros-Dios, J.M., Baysson, H., Bochicchio, F., Deo, H., Falk, R., Forastiere, F., Hakama, M., Heid, I., Kreienbrock, L., Kreuzer, M., Lagarde, F., Mkelinen, I., Muirhead, C., Oberaigner, W., Pershagen, G., Ruano-Ravina, A., Ruosteenoja, E., Rosario, A.S., Tirmarche, M., Tomsek, L., Whitley, E., Wichmann, H.E. and Doll, R. (2005) Radon in Homes and Risk of Lung Cancer: Collaborative Analysis of Individual Data from 13 European Case-Control Studies. British Medical Journal, 330, 223-226.
https://doi.org/10.1136/bmj.38308.477650.63
has been cited by the following article:
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TITLE:
Optimizing Sampling, Sample Processing and Analysis Methods for Radon (222Rn) in Water by Liquid Scintillation Counting
AUTHORS:
Uttam K. Saha, Michael E. Kitto, Dana R. Lynch, Anchal Bangar, Pamela R. Turner, Gabrielle Dean, Leticia S. Sonon
KEYWORDS:
Mineral Oil, Opti-Fluor, Proficiency Test (PT), Radon (222Rn), Liquid Scintillation
JOURNAL NAME:
American Journal of Analytical Chemistry,
Vol.9 No.1,
January
12,
2018
ABSTRACT: Throughout the United States, laboratories use different sampling methods
(“Direct Fill” vs. “Submerged Bottle” methods), sample preparations (“Simultaneous
Drawing” vs. “Separate Drawing”), scintillators (“Mineral Oil” vs. “Opti-Fluor”),
volume of water plus scintillator in the cocktail (“8 mL plus 8 mL” vs. “10 mL plus
10 mL”), and liquid scintillation counting assays (“Full Spectrum: 0 - 2000 keV” vs. “Region of
Interest: 130 - 700 keV”) for analyzing radon (222Rn) in water. We compared these
and few other variables on the recovery of radon from two “Proficiency Test (PT)”
samples and four “Household Well Water” samples from Georgia. The “130 - 700 keV” assay had significantly
higher radon recovery than the “0 - 2000 keV” assay. The “Direct
Fill” sampling produced significantly lower radon recovery than the “Submerged Bottle”
sampling. “Simultaneous Drawing” of both scintillator and water sample yielded higher
radon recovery than “Separate Drawing”. Air bubble in the samples resulted in significant
loss of radon gas; and such loss became greater as the air bubble was larger. A
“10 mL scintillator + 10 sample” combination appeared better than “8 mL scintillator
+ 8 mL sample”. Mixing scintillator and sample in the laboratory, when compared
with doing it on-site, was found superior for better results and practicality of
testing radon in private well waters. “Mineral Oil” scintillator provided higher
radon activity than “Opti-Fluor”. However, in 10 consecutive measurements of the
two proficiency test (PT) samples at 60 days interval (i.e., with full ingrowing), “Mineral Oil” overestimated the radon activity
compared to the predicted/assigned value in most cases, whereas “Opti-Fluor” invariably
produced results close to the predicted/assigned value. There were noticeable temporal
variations in both radon and uranium concentrations in the study wells; nevertheless,
uranium and radon concentrations had good positive correlation. Despite this, the
use of uranium concentration over 30 ppb (the MCL of uranium in drinking water) as a trigger for recommending test
for radon in well water remains questionable because there may be the safe level of uranium but
unsafe level of radon in a well and vice versa.
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